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Temperature-dependent volume nucleation rate coefficients for supercooled water droplets, JV(T), are derived from infrared extinction measurements in a cryogenic laminar aerosol flow tube using a micr...
In this study we introduce a new flow tube suitable for binary and ternary homogeneous nucleation studies. The production of sulfuric acid and water vapor mixture, the experimental setup and the metho...
During the ASTAR (Arctic Study of Tropospheric Aerosol and Radiation) campaign nucleation mode particles (4 to 13 nm) were quite frequently observed at altitudes below 4000 m. However, in the upper fr...
This study presents a comprehensive ice cloud formation parameterization that computes the ice crystal number, size distribution, and maximum supersaturation from precursor aerosol and ice nuclei. The...
Binary heterogeneous nucleation of water-succinic/glutaric/malonic/adipic acid on nanometer-sized particles is investigated within the frame of classical heterogeneous nucleation theory. Homogeneous n...
We present the hypothesis of homogeneous nucleation of ice nano-particles in the polar summer mesosphere. The nucleation of condensed phase is traced back to the first step on the formation pathway, w...
We present a parameterization of cirrus cloud formation that computes the ice crystal number and size distribution under the presence of homogeneous and heterogeneous freezing. The parameterization is...
The nucleation of NAD and NAT from HNO3/H2O and HNO3/H2SO4/H2O solution droplets is investigated both theoretically and experimentally with respect to the formation of polar stratospheric clouds (PSCs...
Number concentrations and mean sizes of ice crystals and derived microphysical and optical properties of subvisible cirrus clouds (SVCs) formed by homogeneous freezing of supercooled aerosols are inve...
We investigate theoretical, laboratory, and atmospheric evidence for a recently proposed hypothesis: homogeneous ice nucleation initiates at the surface, not in the volume, of supercooled water drops....
In a recent published paper Knopf et a1. (2002) have suggested that the homogeneous freezing behavior of stratospheric aerosols, under polar winter conditions, can be simulated experimentally in large...
Box model simulations of an uplifting and adiabatically cooling cloud of aerosol have been performed in order to study the transition between cirrus formation dominated by homogeneous nucleation of ic...
The homogeneous freezing of supercooled H2SO4/H2O solution droplets was investigated in the aerosol chamber AIDA (Aerosol Interactions and Dynamics in the Atmosphere) of Forschungszentrum Karlsruhe. 2...
The homogeneous freezing of supercooled H2SO4/H2O aerosols in an aerosol chamber is investigated with a microphysical box model using the activity parameterization of the nucleation rate by Koop et al...
Laboratory experimental results of iodine oxide nucleation are presented. Nucleation was induced following UV photolysis of CF3I or CH2I2 in the presence of excess ozone. Measurements were performed i...

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