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青岛大气中HNO3、HNO2、NH3及PM2.5中氮组分的浓度特征和气-粒平衡关系
硝酸气体 亚硝酸气体 氨气
2014/12/20
研究PM2.5中NO3-、NO2-、NH4+及其气态前体物HNO3、HNO2、NH3的浓度特征和气-粒平衡关系,对深入认识PM2.5的来源及控制因素具有重要意义.因此,本文利用2012年6—7月在青岛采集的denuder和PM2.5大气样品,分析了其中气态和颗粒态氮组分的浓度.结果发现,青岛大气中HNO3、HNO2和NH3浓度分别为(0.80±0.79) μg·m-3、(0.49±0.59) μg...
Gas-particle interactions above a Dutch heathland: III. Modelling the influence of the NH3-HNO3-NH4NO3 equilibrium on size-segregated particle fluxes
Gas-particle interactions Dutch heathland NH3-HNO3-NH4NO3 equilibrium particle fluxes
2009/3/2
Micrometeorological measurements of size-segregated particle number fluxes above Dutch heathlands and forests have repeatedly shown simultaneous apparent emission of particles with a diameter (Dp)<0.1...
Gas-particle interactions above a Dutch heathland：I. Surface exchange fluxes of NH3, SO2, HNO3 and HCl
Gas-particle interactions Dutch heathland NH3 SO2 HNO3
2009/2/27
A field measurement campaign was carried out over a Dutch heathland to investigate the effect of gas-to-particle conversion and ammonium aerosol evaporation on surface/atmosphere fluxes of ammonia and...
Growth of upper tropospheric aerosols due to uptake of HNO3
upper tropospheric aerosols HNO3
2009/2/24
The effect of nitric acid on the equilibrium size distributions of upper tropospheric aerosols is calculated as a function of relative humidity. It is shown that HNO3 concentrations above a few tenths...
Heterogeneous conversion of NO2 and NO on HNO3 treated soot surfaces: atmospheric implications
NO2 NO HNO3 soot surfaces atmospheric implications
2009/1/23
For the treatment of soot by pure HNO3 only reversible uptake with a surface coverage of ~1-2x1014 HNO3 cm-2 was observed for HNO3 mixing ratios in the range 250-800ppbv. Only for higher HNO3 mixing r...
On the ability of chemical transport models to simulate the vertical structure of the N2O, NO2 and HNO3 species in the mid-latitude stratosphere
chemical transport models vertical structure N2O HNO3 species mid-latitude stratosphere
2009/1/7
In this paper we study the impact of the modelling of N2O on the simulation of NO2 and HNO3 by comparing in situ vertical profiles measured at mid-latitudes with the results of the Reprobus 3-D CTM (T...
Nitric acid (HNO3) is one of the key products that are operationally retrieved by the European Space Agency (ESA) from the emission spectra measured by the Michelson Interferometer for Passive Atmosp...
Impact of the new HNO3-forming channel of the HO2+NO reaction on tropospheric HNO3, NOx, HOx and ozone
HNO3-forming channel HO2+NO reaction tropospheric HNO3 NOx HOx ozone
2008/11/13
We have studied the impact of the recently observed reaction NO+HO2→HNO3 on atmospheric chemistry. A pressure and temperature-dependent parameterisation of this minor channel of the NO+HO2→NO2+OH reac...
Observations of HNO3, ΣAN, ΣPN and NO2 fluxes: evidence for rapid HOx chemistry within a pine forest canopy
HNO3 HOx chemistry forest canopy
2008/11/13
Measurements of exchange of reactive nitrogen oxides between the atmosphere and a ponderosa pine forest in the Sierra Nevada Mountains are reported. During winter, we observe upward fluxes of NO2, and...